The invention discloses a high-strength wear-resistant gray cast iron and an inoculation process thereof, and relates to the technical field of wear-resistant gray cast iron inoculation. The present invention includes the weight ratio of each component as follows: C: 4.28%, Cr: 0.05%, Mn: 1.57%, Si: 0.38%, Ti: 0.38%, P<0.02%, S<0.15%, B: 0.67 %, Ni: 0.96%, Mo: 0.082%, V: 0.11%, Sn: 0.09%, and the rest is Fe. The present invention adopts inoculation treatment in front of the furnace and in the ladle during the manufacture of gray cast iron, mixes and bakes the silicon-barium inoculant and rare earth ferrosilicon to 100-150°C, and then adds them into the molten iron along with the flow of the tapping trough for follow-up Flow inoculation treatment, promotes nucleation, inhibits growth, refines grains, promotes graphitization, reduces whitening tendency; improves the uniformity of the section, improves the mechanical properties of gray cast iron, and improves the wear resistance of gray cast iron.