The invention discloses a preparation method and a production device of large-particle spherical glass, a gas-material co-spraying balling process is adopted, in the balling process of the glass, the glass does not make contact with other materials, the surface is smooth, and secondary treatment and cleaning are not needed. And the outlet of a high-temperature furnace adopts a trumpet-shaped flame structure, so that the static pressure of a high-temperature section is increased on the basis of ensuring the low-temperature kinetic energy of the frit, and the high-temperature separation of gas and solid glass balls is strengthened while the frit is fully heated. Oxygen-enriched combustion flames are adopted, so that the rigidity of the flames is improved, the atmosphere in the combustion process is ensured, and the color of the glass is stable. And a gas and furnace temperature linkage control technology is adopted, so that the product quality is ensured, and the production cost is reduced. A furnace body structure step-by-step heat preservation technology is adopted, so that the high temperature is not reduced, the low temperature is not increased, meanwhile, the cost is saved, and the production efficiency is improved. And the top cover is cooled by water, so that the service life of the equipment is fully prolonged while environmental protection is realized.