The invention discloses a method for preparing Al-Pd-Fe two-dimensional quasicrystal particles. The Al-Pd-Fe quasicrystal comprises 70-75% of Al, 10-25% of Pd and 5-15% of Fe. The method comprises: fully and uniformly mixing high-purity Al powder, Pd powder and Fe powder through a mortar, uniformly distributing the mixed metal powder in a graphite abrasive cavity, pre-pressing the mixed metal powder through a mold tableting machine, keeping 1-2MPa for 60-100s, coating a graphite crucible with a carbon felt, orderly placing a carbon paper, a large graphite block, a carbon paper, a small graphite cushion block, the prepared graphite crucible, a small graphite cushion block, a carbon paper, a large graphite cushion block and a carbon paper in a pressure chamber of SPS, carrying out compression, carrying out heating to 1000 to 1100 DEG C under sintering pressure of 50MPa, keeping the temperature for 10-20min and carrying out furnace cooling to the room temperature. The method has simple processes and strong operability, utilizes conventional equipment, has small time consumption, is free of raw material treatment and directly uses mixed raw materials to synthesize the two-dimensional quasicrystalline phase.