The invention discloses a wind power generation high-voltage direct current grid-connected system based on an open coil structure. The wind power generation high-voltage direct current grid-connected system comprises a permanent magnetism synchronous wind driven generator, two generator side converters, two direct current boosters and a controller, wherein the permanent magnetism synchronous wind driven generator is of the open coil structure, and each direct current booster is composed of an electric reactor, an inverter, a transformer and a rectifier in a sequentially connected mode. According to the wind power generation high-voltage direct current grid-connected system based on the open coil structure, the open coil permanent magnetism synchronous wind driven generator is used, the two double-level three-phase controllable full-bridge converters are used for controlling the permanent magnetism synchronous wind driven generator, three-level modulation is achieved, voltage stress of converter capacity and voltage stress of switching elements are reduced, and system cost can be reduced. The wind power generation high-voltage direct current grid-connected system based on the open coil structure is simple in structure, low in cost and high in operational efficiency. The invention further discloses a method for controlling the system. According to the method, the better PWM technology of the vector control strategy is used, therefore, current harmonic contents inside the generator can be reduced, and the generator can better operate.