The invention discloses an intelligent gas supply control system for a liquefied natural gas (LNG) vehicle. The system comprises an intelligent control unit, a hydraulic oil tank, a hydraulic oil pump, an LNG infusion pump, an LNG bottle, a carburetor, a valve set, a hydraulic pressure sensor, a carburetor back fuel gas temperature sensor, a buffer tank, a buffer tank fuel gas pressure sensor and a buffer tank fuel gas temperature sensor. The intelligent control unit collects the state information of an engine, an LNG bottle liquid level meter as well as all the sensors mounted in the system; the pressure and flow direction of a hydraulic system are controlled by controlling movement of the valve set to drive the LNG infusion pump to pump out LNG liquid from the LNG bottle; and according to the state requirement of the whole vehicle, the working frequency of the LNG infusion pump is controlled, the target pressure of the buffer tank is adjusted or maintained to meet the requirement of the whole vehicle for gas supply, and additionally, the intelligent control unit has the function of fault diagnosis and treatment, so that the effect that the intelligent gas supply control system achieves the safe, efficient, intelligent and energy-saving gas supply purpose is guaranteed.