The invention relates to the field of math teaching tools and specifically to a mathematical probability operation device for a coin-toss experiment and a control system of the mathematical probability operation device. The operation device comprises a machine body, a coin ejecting device, a coin receiving device and a coin returning device. The machine body comprises a stand, support plates, a bottom plate, a front baffle plate and a rear baffle plate, and a separator plate. The coin ejecting device comprises six coin ejectors. Each coin eject comprises a coin ejecting plate, a coin supporting plate, a first spring, a first ejecting column, a first iron block, and a first electromagnet. The coin receiving device comprises a rodless push plate cylinder, a sliding block, a coin receiving plate, a limiting plate, a rotating plate cylinder, a connecting base, a rotating wheel and a slide rail. The coin returning device comprises a left returning device and a right returning device. The control system comprises a programmable controller, a sensor unit, an air pressure unit and a servo controller. The operation device and the control system can satisfy the needs of frequent mathematical probability experiments and enable students to learn the process of coin-toss experiments directly.