The invention discloses an antiferromagnetic
metal single crystal with a three-dimensional stacking ordered structure and a preparation method of the antiferromagnetic
metal single crystal. The preparation method comprises the following steps: uniformly mixing Fe
powder, Co
powder, Ge
powder and Te powder, and then loading the mixture into a
quartz tube together with a
transport agent; putting the sealed
quartz tube into a double-temperature-zone tubular furnace for calcining to obtain the antiferromagnetic
metal single crystal; a unit
cell of the antiferromagnetic metal single
crystal is formed by stacking a plurality of layer structures layer by layer, and each layer structure is provided with two Te
layers, a Ge layer and a Fe / Co layer, wherein the Ge layer and the Fe / Co layer are respectively positioned between the two Te
layers; the plurality of layer structures are grouped in pairs to form a plurality of layer groups which are sequentially stacked, the
two layer structures in the same
layer group are in an AA stacking mode, and the
two layer structures in the two adjacent layer groups are in an ordered staggered stacking mode. The antiferromagnetic metal single
crystal has the characteristics of good cruising
antiferromagnetism, neel temperature higher than
room temperature, three-dimensional stacking ordered structure and the like, and promotes the development of related fields.