The invention discloses a waste mercury recovery and purification device and a use method thereof. The waste mercury recovery and purification device comprises a control mechanism, a vibration sieving mechanism and a filtering and solution storage mechanism. According to the invention, waste mercury solution can be purified through combination and adjustment, thus generation of toxic wastes is reduced, the inventory rate of hazardous wastes is decreased, the cost of experimental materials is reduced, and the usage rate of mercury is increased; the traditional purification method is broken through, and an organic solvent and high-temperature operation or low-temperature operation are not required, thus the purification method is expanded; high-strength polytetrafluoroethylene plastic is used, thus the support strength is ensured, and moreover, the high-strength polytetrafluoroethylene plastic is corrosion-resistant, free from reacting with mercury, light in weight, and convenient to move and carry; and in the invention, a physical sieving method is utilized, and has the advantages of being high in safety, high in purification effect, simple in equipment and method, low in cost, convenient to move, convenient to operate, easy to popularize and use, and the like compared with the existing purification technologies of vacuum distillation, acid-base washing, and the like.