The invention discloses a CO<2> geological storage method and a CO<2> geological storage system. The method comprises the following steps that a CO<2> reservoir stratum and a cover layer are determined according to a geological environment; a CO<2> injection well and a salt water extraction well are excavated, and the CO<2> injection well and the salt water production well both communicate with the CO<2> reservoir stratum; CO<2> is injected into the CO<2> reservoir stratum through the CO<2> injection well, meanwhile, salt water in the CO<2> reservoir stratum is extracted through the salt water extraction well, the pressure of the CO<2> reservoir stratum is reduced, and the pore available space of the CO<2> reservoir stratum is increased; and the CO<2> is stored in the CO<2> reservoir stratum in a sealed mode; According to the method, the salt water extraction well is excavated while the CO<2> injection well is excavated, CO<2> is injected into the CO<2> reservoir stratum through the CO<2> injection well, and meanwhile salt water in the CO<2> reservoir stratum is extracted through the salt water extraction well, so that the pressure of the CO<2> reservoir stratum is reduced and the pore available space of the CO<2> reservoir stratum is increased, and therefore the storage coefficient of the CO<2> reservoir stratum can be remarkably increased, and then the total storage amount of the CO<2> reservoir stratum is increased, namely, the sealing capacity of the CO<2> reservoir stratum is improved.