The invention relates to a purification method of ultra-pure aluminum, comprising the following steps: cleaning and
drying raw refined aluminum, wherein the purity of the selected refined aluminum is at least 4N6, Mg is less than 6ppm, Ti is less than 0.2ppm and Zr is less than 0.2ppm; loading the selected raw refined aluminum into a purification furnace, sealing and vacuumizing the furnace, and heating to 680-750 DEG C by using a gas furnace to melt the
solid raw refined aluminum to form liquid; moving the purification furnace heated to 680-750 DEG C to a
crystal growing furnace which is kept at 660 DEG C inside by a
crystal growing furnace heater, rotating the aluminum liquid of the purification furnace in the
crystal growing furnace heater, and enabling the aluminum liquid inside the purification furnace to self-keep the
crystallization speed at 5-10 cm / h by controlling the heat dissipating capacity of the crystal growing furnace and finishing the
crystallization after 4-6 hours; cooling the crystallized purification furnace, taking out a
crystallization ingot, removing 25-35 percent relative to the
mass of the crystallization from the
tail part of the crystallization
ingot and obtaining a first purified aluminum
ingot; placing the first purified aluminum ingot into the purification furnace again, and repeating purification until the aluminum ingot reaching the required precision is obtained.