The invention belongs to the technical field of physical measurement, and in particular relates to a magneto-optic Kerr effect and magnetocrystalline anisotropy field measurement system and a measurement method. The measurement system comprises a magnet control part and a laser detection part. The magnet control part mainly comprises a magnet bracket, power supplies, an ADDA (analog-digital and digital-analog) card and a computer, wherein the computer respectively controls the size and the direction of output current of the two power supplies through the ADDA card, and respectively controls the size and the direction of magnetic fields so as to obtain a required resultant magnetic field; and the laser detection part is composed of a laser device, a polarizer, a polarization analyzer, a photoelectric detector, an ADDA card and a computer, wherein laser emitted by the laser device is projected to the photoelectric detector after being filtered by the polarizer and the polarization analyzer, signals are transmitted to the computer after being converted by the ADDA card, and then Kerr signals of a detection point are obtained. According to the measurement system and the measurement method, the mechanical vibration can be eliminated, the noise in the measurement can be reduced, the accuracy of the measurement can be increased, and magnetic signals and the magnetocrystalline anisotropy field of a sample can be accurately and efficiently obtained.