The invention relates to a method for producing silicon deoxygenation low-sulfur high-carbon steel through an LF refining double slag method. An electric furnace-LF-VD continuous casting technology isadopted. The method includes the steps that in the electric furnace tapping process, carbon powder is mixed firstly, then a silicon alloy and a manganese alloy are added for conducting deoxygenationalloying treatment, and lime, calcium carbide and aluminum-free refining slag are added for conducting modification treatment; secondly, after an LF enters a station, lime, calcium carbide, silicon iron and aluminum-free refining slag are added into the furnace for making high-alkalinity reducing refining slag; thirdly, low-alkalinity reducing slag is made, and the content of components in moltensteel is adjusted; and fourthly, the LF withdraws from the station after refining, VD and continuous casting processes are conducted in sequence, and the silicon deoxygenation low-sulfur high-carbon steel is obtained. The method is simple, reliable, high in operability and easy to achieve, the production cost of the whole process is reduced, the sulfur removing efficiency is high, the cleanlinesslevel of molten steel is high, the problem that when a non-molten-steel pretreatment sulfur removing process is adopted for producing high-quality silicon deoxygenation low-sulfur high-carbon steel, sulfur removing is difficult is solved well, and therefore the product quality is improved, and the economic benefits of a steel enterprise are increased.