The invention discloses a navigation solution method realized based on an atomic gyroscope navigation system. The method comprises the following steps of S1, constructing coordinate systems for navigation solution, S2, defining navigation parameters including geographic longitude, geographic latitude, geographic height, north speed, east speed, vertical speed and carrier attitude angle, and related physical parameters including platform attitude angle and accelerometer installation misalignment angle, S3, solving the position and the speed of the atomic gyroscope navigation system, and solving the geographic longitude, the geographic latitude, the geographic height, the north speed, the east speed and the vertical speed of the carrier, and S4, calculating the attitude angle of the carrier according to the navigation parameters. According to the atomic gyroscope navigation system and the navigation solution method thereof, a framework of an inertial navigation system for the atomic gyroscope and the navigation solution method of the atomic gyroscope are provided for the first time, the application of the atomic gyroscope in the inertial navigation system is expanded, the error value between each piece of navigation data resolved by the navigation solution steps and actually measured navigation data is small, the precision is high, and the effectiveness and the practicability are high.