The invention discloses a double-layer ball milling device for high-purity quartz sand processing in the technical field of high-purity quartz sand processing. The double-layer ball milling device comprises a base, an outer cylinder, an inner cylinder and a storage box, wherein a driving assembly is arranged on the base, and the base is connected with the inner cylinder and the outer cylinder through the driving assembly; the storage box is connected with a feeding pipe, and a sealing assembly is arranged in the feeding pipe; and the sealing assembly is correspondingly connected with a rotating wheel on the inner cylinder. According to the double-layer ball milling device, the inner cylinder is rotated through the driving assembly, so that quartz sand is subjected to primary ball milling through a ball milling ball, and enters the outer cylinder through sieve holes, and meanwhile, intermittent discharging is realized through the rotating wheel and the sealing assembly; the outer cylinder is enabled to swing in a reciprocating mode through a rotating disc and rotating rods, and the quartz sand is subjected to secondary grinding; and a connecting shaft is separated from the rotatingrods through an electromagnet, the outer cylinder is turned over until a screen is downward, so that discharging is facilitated, the connecting shaft is connected with the corresponding rotating rod again, and as a result, the outer cylinder swings and drives the quartz sand to move at the screen, and the screening and discharging effect is improved.