The present invention relates to a device and method for capturing
carbon dioxide from the
atmosphere based on an
air separation unit, and relates to the technical field of CO2 capture. The device comprises an
air filtration device, a compressor unit, a cooling device, a
molecular sieve adsorption group, a gas buffer device, an amine absorption device, a
liquid storage device, a first heating device, an amine regeneration device, and a
carbon dioxide storage device, which are connected in sequence. The post-adsorption
gas phase outlet of the
molecular sieve adsorption group is connected to the air inlet of the
air separation unit. The first air outlet of the
air separation unit is connected to the cooling device via a liquid cooling device and a
refrigeration device in sequence. The second air outlet of the air separation unit is connected to the desorbed gas inlet of the
molecular sieve adsorption group via a second heating device. The device provided by the present invention uses the molecular
sieve adsorption group to adsorb CO2. The adsorbed gas enters the air separation unit to produce high-purity
nitrogen and
liquid oxygen. The CO2-containing gas enters the amine absorption
tower and the amine regeneration
tower to obtain high-purity CO2, thereby achieving low-
energy consumption and low-waste
air capture and production of CO2.