The invention discloses a method of quickly calibrating an oblique redundant strapdown inertial navigation system. The method comprises the following steps of: 1, describing a mounting misalignment angle of the oblique RSINS (Redundant Strapdown Inertial Navigation System), and giving a calibrating measurement equation; 2, designing a calibrating scheme of the oblique RSINS; and 3, constructing a calibrating simulation platform of the oblique RSINS, and verifying accuracy of the calibrating method by utilizing the simulation platform. The method, provided by the invention, is capable of quickly calibrating the oblique RSINS on the basis of a tri-axial position/speed turntable, calibrating parameters, such as zero offsets, scale factors and mounting misalignment angles of a redundant accelerometer and a gyro, are calibrated by utilizing a four-position method and a three-position rotating method, and accuracy of the calibrating method can be verified by utilizing the simulation platform. The method, provided by the invention, has the advantages of high calibration precision, simple operation, capability of meeting quick calibration requirements of the oblique RSINS at low and middle precisions, and better engineering application value.