The invention discloses a preparation method of a high-strength graphene material. The preparation method comprises the following steps of: taking raw materials of graphite, diester phthalate, methylisobutyl ketone, trinonyl phenyl ester phosphite, SEBS (Styrene-Ethylene-Butylene-Styrene), fibrilia, calcium stearate, polyvinylidene fluoride, zinc oxide, titanium dioxide, PVC (polyvinyl chloride),CPE (Chlorinated Polyethylene), SMA (Stone Mastic Asphalt), graphene oxide and a crosslinking agent, uniformly mixing, plastically granulating, and then calcining to obtain the high-strength graphenematerial. The preparation method disclosed by the invention has the beneficial effects that the raw materials are wide in source and low in cost, the Rockwell hardness is 110-150, the high-strength graphene material can be self-extinguished after leaving from a fire, and the thermal deformation temperature is increased by 20-30%; the elongation at break is up to 300-500%, and the tensile strengthis 80-120MPa; the permanent compression deformability is good, the energy density is high, the conductivity is good and the thermal conductivity is 35-55W/(m.k); the high-strength graphene material is good in printing electrode property, is high-efficiency and energy-saving and can be accurately prepared; all the components generate a synergistic effect, and the notched impact strength is 70-110J/m; the high-strength graphene material is convenient in use, good in thermal conductivity and simple in process, and can be widely used.