The invention belongs to the technical field of daily cosmetics, and relates to novel cleansing milk containing a liquid crystal structure and a preparation method of the novel cleansing milk. The preparation method of the novel cleansing milk comprises the steps that lauramide propyl betaine, potassium lauryl ether phosphate and the like are added with water for being heated and dissolved and a dissolved dimeric amino acid salt compound liquid crystal emulsifier is added, uniform stirring is carried out, then plant essential oil is added, a crylic acid (ester) cross-linked polymer is added after temperature reduction, polyquaternium-43, citric acid and the like are added when system temperature is reduced to 35-45 DEG C, pH is controlled at 6.5-7.5, and after physical and chemical indexespass the inspection, discharging is carried out to obtain the novel cleansing milk containing the liquid crystal structure. The preparation technology is simple, the liquid crystal emulsifier and a phosphate ester surfactant system act to rapidly form a large number of crystal lattice, the lattice can be wrapped with added grease through simple stirring, a foam state is not affected, the good refreshing and foam effects can be brought, the effects of comfort, no stimulation, no tightness and the light after washing are achieved, and all-around value ideas are brought for cleansers.