The invention provides a method for preparing a titanium nanosheet / graphene-based fiber membrane, comprising the following steps: preparing a pre-stripping dispersion of titanium powder, preparing a mixture of titanium powder and graphene oxide, and preparing a titanium nanosheet / graphene oxide Dispersion, spinning and finishing. The preparation method of the titanium nanosheet / graphene-based fiber membrane of the present invention can not only assist the stripping of titanium powder into titanium nanosheets, but also help the mixing of titanium nanosheets and graphene oxide by adding graphene oxide in the preparation process of titanium nanosheets . In the spinning process, titanium nanosheets, graphene and carbon black are further loaded onto the fiber, which has the advantages of large specific surface area, strong infrared radiation, high thermal conductivity, good flexibility, and remarkable bending resistance. The PAN polymer makes the fiber have the advantages of high mechanical strength, medium and high temperature resistance, etc. The invention also provides a titanium nanosheet / graphene-based fiber membrane.