The invention relates to a method for reinforcing a brick-concrete structure by utilizing an angle steel frame, belonging to the anti-earthquake reinforcement field. According to the method disclosed by the invention, a reliably connected steel frame formed by double-angle steel can replace a ring beam and a structural column, and field bolt assembly connection through factory pre-fabricated components can be realized, thus the safe, environment-friendly and green construction is realized; simultaneously, angle steel, a wall and a pre-fabricated floor slab are connected by bolts and epoxy resin, and the double-angle steel is also can be used as a round hole plate end part support, so that the connection reliability of the pre-fabricated floor slab and the wall is ensured, double functions of the ring beam and a supporting beam are exerted, reinforcement workload and cost are saved, and the original structure and reinforcement components mutually and cooperatively work. According to the method for reinforcing the brick-concrete structure by utilizing the angle steel frame, disclosed by the invention, the binding-type reinforcement construction speed is fast, and the reinforcement construction is safer, so that the method is very suitable for residential buildings.