The application discloses a flexible brain-computer interface composite device and a preparation method thereof. The flexible brain-computer interface composite device comprises a flexible substrate, a bottom
electrode layer, a functional film layer and a top
electrode layer which are arranged in a stack; the functional film layer comprises a first epitaxial layer, a light-emitting layer and a second epitaxial layer which are arranged in a stack from the bottom
electrode layer to the top electrode layer; one of the first epitaxial layer and the second epitaxial layer is an n-type doped
semiconductor material, and the other is a p-type doped
semiconductor material; and the material of the light-emitting layer is
indium gallium nitride. The application can combine the functions of collecting brain electrical signals, emitting
light stimulation signals and providing energy for the device into the same device structure, so that the volume of the brain-computer interface device can be reduced and the integration degree can be improved.