The application provides an online in-situ low-temperature high-pressure ultrafast
spectroscopy device, a
system and a method thereof. The high-pressure device comprises a
cold shield with an optical window, a
metal ring, a
gasket, a first pressurized air bag, a second pressurized air bag, a pressurized
metal column,
a diamond anvil
cell, a first temperature sensor, a second temperature sensor, a heat-conducting base, a
cryostat and a
gas pressure controller. The online in-situ pressure calibration and imaging
system comprises a
continuous light laser, the high-pressure device, online in-situ pressure optical components and an online in-situ pressure imaging
system. The low-temperature high-pressure ultrafast pump-probe system comprises a
femtosecond laser, the online in-situ pressure calibration and imaging system, pump-probe optical components and a pump-probe imaging system. The application realizes temperature regulation at 6-325K under
high pressure with double air bag pressure regulation, realizes online in-situ free pressure regulation at low temperature, and realizes continuous regulation with an accuracy of 0.1GPa in the
pressure range of 0-80GPa, and realizes online in-situ low-temperature high-pressure ultrafast
spectroscopy and ultrafast dynamics measurement.