The present invention relates to the field of transient dynamics and catalytic surface and interface research, and provides a pump-probe TAP instrument. The pump-probe TAP instrument provided in the present invention comprises a sample injection pulse
system, a micro-reactor, a
liquid nitrogen cooling
system, a
mass spectrometry
system, and a vacuum system; the vacuum system comprises a first vacuum cavity, a second vacuum cavity and a
vacuum pump group which are connected in sequence, and the side wall of the first vacuum cavity is provided with a vacuum gauge having a working end extending into an inner cavity of the first vacuum cavity; the
liquid nitrogen cooling system comprises an annular
liquid nitrogen cavity provided in the first vacuum cavity; the sample injection pulse system comprises a pulse
flange provided on the top of the first vacuum cavity, a first pulse valve and a second pulse valve are provided in the pulse
flange, and an included angle α is formed between the first pulse valve and the second pulse valve; the pulse
flange is also provided with a
condensed water piping channel for accommodating
condensed water piping; the micro-reactor is provided at the bottom of the pulse flange, the pulse flange is further provided with a pulse channel, the first pulse valve and the second pulse valve are connected to the top of the micro-reactor by means of the pulse channel, and the micro-reactor is suitable for loading a sample; the
mass spectrometry system comprises a
mass spectrometer, the mass
spectrometer is provided on the side wall of the first vacuum cavity, and a mass
spectrometer filament of the mass spectrometer extends to the center of the first vacuum cavity; and the bottom of the micro-reactor is further provided with an extension tube extending towards the mass spectrometer filament and located above the mass spectrometer filament. By means of the arrangement, the present invention can realize experiments involving continuous pulses, intermitt