The invention relates to a method for preparing a high-purity spraying-free coating at the bottom of an ingot casting single crystal. The method comprises the following steps: grinding fused quartz particles and deionized water in a ball mill, taking the resulting product out, adding the resulting product in a dispersion machine, adding silica sol, fused quartz powder, fused quartz powder and a high-purity ceramic binder, and stirring the mixture to form slurry A; adding fused quartz particles and deionized water into the ball mill for milling, taking the resulting product out, adding the resulting product into a stirrer, adding silica sol and fused quartz powder, and stirring the mixture to form slurry B; adding fused quartz particles and crystalline quartz in the ball mill for milling, taking the resulting product out, and mixing quartz slurry, silica sol, a binder and water to form slurry C; adding silicon nitride and deionized water to the stirrer, adding a silicon nitride sintering aid, silica sol and a high-purity binder, and fully stirring the mixture to form slurry D; and sequentially manufacturing a bottom lining flat layer, a rough loose layer, a quartz compact isolationlayer and a silicon nitride compact isolation layer. The method can effectively reduce a red area at the bottom of the ingot casting single crystal, and can reduce the proliferation of dislocation andother defects.