A wear resistant multilayer overlay includes a first layer on at least a surface of an article, and a second layer metallurgically bonded to at least a portion of the first layer. The first layer includes a first continuous metallic matrix and at least one of first hard particles, blocky diamond particles, non-blocky diamond particles, TSP diamond, cubic boron nitride particles, and PCD compacts embedded in the first continuous metallic matrix, wherein the first hard particles are at least one of transition metal carbide particles and boron nitride particles. The second layer includes a second continuous metallic matrix and at least one of second hard particles, blocky diamond particles, non-blocky diamond particles, TSP diamond, cubic boron nitride particles, and PCD compacts, embedded in the second continuous metallic matrix, wherein the second hard particles are at least one of transition metal carbide particles and boron nitride particles. Related methods and articles of manufacture also are disclosed.