The invention relates to the technical field of bedding textile articles, and particularly discloses a dandruff-removing and hair-cleaning pillow towel fabric. The pillow towel fabric is prepared from: bamboo fiber, linen fiber, aloe fiber, silk fiber and dandruff-removing modified polyester fiber. Two sides of the pillow towel fabric are coated with a dandruff-removing medicine liquid layer. The dandruff-removing modified polyester fiber is prepared from: polyethylene glycol terephthalate master batches, polymethyl methacrylate master batches, nano silicon dioxide, borax, pearl nacre powder, a dandruff-removing plant extract powder, a vinyl silane coupling agent, and viscose fiber. The dandruff-removing plant extract powder is prepared from: sapindus delavayi, salvia miltiorrhiza, polygonum multiflorum, fructus cnidium monnieri, leaves of cacumen biotae, black sesame, lily flower, thyme, white vinegar, etc. The pillow towel fabric can improve blood circulation of head, improve ecological balance of microflora of head, improve growth of hairs and inhibit generation of dandruff. The fiber raw materials have good breathability and moisture absorption performance, so that accumulation of sweat and heat on head is avoided so as to guarantee an excellent sleep environment.