The invention discloses a method for manufacturing a carbon molecular sieve with a plant nutshell, which sequentially comprises the following steps: a, crushing the plant nutshell into powdery material; b, drying and grinding the powdery material to obtain micro-powdery material; c, mixing and kneading the micro-powdery material with adhesives in a kneader; d, placing the kneaded material into a bar extruding machine for formation; e, placing the formed material into a converter for carbonization; and f, depositing the carbonized material with carbon to obtain a finished carbon molecular sieve. By adopting the method, the problem of environment pollution caused by the carbon molecular sieve process can be solved effectively, and the environment protection can be facilitated. Meanwhile, the finished carbon molecular sieve is manufactured with the plant nutshell sequentially via crushing, drying, grinding to produce the micro powder, placing of the micro powder along with the adhesives into the kneader, formation, carbonization and surface carbon deposition to obtain the finished carbon molecular sieve. Waste is fully utilized to manufacture high-value products, the manufacturing cost of the carbon molecular sieve is reduced, the process is simple, and industrialization can be realized easily.