The invention belongs to the field of garden and park landscaping, and particularly relates to a processing reagent of a plant material for landscape decoration, and a preparation method thereof. Theprocessing reagent is prepared from the following raw materials: polyacrylate emulsion, titanium dioxide, water-based acrylic resin emulsion, ethanol, an organic silicon defoamer, a dispersing and thickening agent, a film forming auxiliary agent, a wetting agent, a multifunctional aid, a preservative, a concentrated organic dye, water-based essence and water. According to the invention, the raw materials used in the formula of the plant material processing reagent for landscape decoration are non-toxic and meet the requirements of the international environmental protection standard; the reagent is simple in processing process and low in raw material cost; and the plant material processed by adopting the reagent is soft in texture, fresh in odor, rich in elasticity in touch, bright and lasting in color and luster, has the characteristics of uniform coloring, good color fastness, water resistance, mildew resistance, abrasion resistance and the like, and can be used for processing commonplant materials such as herbs, woody plants, cladonia rangiferina, moss and the like, and the processed plant material is widely applied to various indoor and outdoor landscape decoration projects.