The invention provides a preparation method for titanium dioxide/carbon nanotube composite nanosheets, and relates to the composite nanosheets. The preparation method comprises the following steps: adding a titanium source into deionized water, performing stirring in an ice water bath, adding an alkaline solution, performing a reaction to generate a white precipitate, performing centrifugation toremove a supernatant liquid, performing washing by using water, dispersing the white precipitate into water, adding hydrogen peroxide until the solution is yellow and transparent, adding deionized water for dilution to obtain a titanium peroxide complex aqueous solution, and storing the aqueous solution in a refrigerator for standby application; dispersing the carbon nanotubes into a nitric acid solution, performing reflux treatment, performing centrifugal washing, and dispersing the carbon nanotubes into deionized water; mixing the titanium peroxide complex aqueous solution and the carbon nanotube dispersion liquid, performing stirring, and allowing the stirred material to stand for aging; and freezing the mixed solution obtained after stand aging, performing drying to remove water to obtain a precursor of bulk-shaped dried titanium dioxide/carbon nanotube composite nanosheets, and performing calcination to obtain the titanium dioxide/carbon nanotube composite nanosheets. The titaniumdioxide/carbon nanotube composite nanosheets provided by the invention have a porous two-dimensional laminated structure.