The invention relates to a silicone iron zinc coagulant and a preparation method thereof, relating to an inorganic polymer coagulant and a preparation method thereof. The invention solves the affection of weak adaptability to low temperature and low turbidity water quality, low turbidity removal rate, residual chroma and fast hydrolysis of the existing molysite coagulant, and the problems of complicated preparation process, high cost of raw materials and long time consuming, and production of second pollution to environment. The silicone iron zinc coagulant is prepared by sodium silicate, dilute sulphuric acid solution, sodium bicarbonate, ferrous sulfate, zinc sulfate and an antioxidant. The preparation method comprises the following steps of: 1. weighing raw materials; 2. preparing clustering silicic acid solution; 3. preparing the clustering ferrosilicon zinc solution and 4. adopting a reverse contact type spray drying method or cocurrent flow contact type spray drying method to dry the clustering ferrosilicon zinc solution, thus obtaining the clustering ferrosilicon zinc coagulant. The product has the advantages of being suitable for low temperature and low turbidity water quality, more than 99 percent of the turbidity removal rate, no residual chroma and being not easy to be hydrolyzed, low preparation cost, simple method and no pollution in preparing process.