The invention discloses a preparation method for a high-hardness manganese-iron alloy material. The preparation method comprises the following steps: S1, Fe is added into a smelting furnace and is heated to be completely melted; S2, Mn, Cr, Zr, Mo, Cd, W, V, graphite, diamond, WC, Cr2B, La2O3, Nd(OH)3, Eu2O3,Yb2O3, PrCl3, PrSi2, YSi2 and TbN are added into the Fe melted in the S1, and are uniformly mixed with the melted Fe to obtain an alloy melt; S3, the alloy melt in the S2 is refined, and a refining agent is added in the refining process; S4, the alloy melt refined in the S3 is cast to obtain a casting; and S5, the casting cooled in the S4 is tempered and cooled to obtain the alloy material. According to the preparation method for the high-hardness manganese-iron alloy material, by adding Cr and rare earth elements, the manganese-iron alloy is high in strength and good in toughness and wear resistance, and the comprehensive performance of the copper alloy is greatly improved.