A method for prepare a high-adhesiveness water-borne polymer coated membrane comprise uniformly mixing polymer powder, dispersant, adhesive, thickener, surfactant and deionize water to obtain polymercoated slurry, mixing that polymer powder, dispersant, adhesive, thickener, surfactant and deionized water to obtain polymer coated slurry, and mixing the polymer powder, dispersant, adhesive, thickener and deionized water. The obtained polymer coating slurry is coated on a polyolefin film and dried to obtain a coated diaphragm crude product; The obtained coated diaphragm crude product is immersedin a modified liquid, and the modified coated diaphragm is obtained by rolling the coated diaphragm in the modified liquid; The obtained modified coating diaphragm is dried to obtain a highly adhesive aqueous polymer coating diaphragm. The high-adhesion waterborne polymer coated diaphragm prepared by the invention remarkably improves the adhesion of the coated diaphragm, avoids the powder dropping phenomenon, is favorable for subsequent processes such as slitting and core winding, and simultaneously remarkably improves the comprehensive performance of the lithium ion battery diaphragm.