The invention provides a binary rare earth organic framework crystal material. The chemical formula of the binary rare earth organic framework crystal material is [Me2NH2][EuxTb1-xL(H2O)4], wherein x is greater than 0 and less than or equal to 5; Me represents methyl; L represents an organic ligand formed by pyridine-2,6 m-phthalic acid; crystals belong to an orthorhombic system, the space group is Pnma, and the cell parameters are as follows: a=8.500 to 8.506 Angstrom, b=17.28 to 17.35 Angstrom, and c=12.05 to 12.15 Angstrom; alpha is equal to 90, beta is equal to 90, gamma is equal to 90, and Z is equal to 4. The binary rare earth organic framework crystal material is extremely high in heat stability and air stability, and can be used for temperature detection within a wide range of 77K to 450K; the temperature range covers a low temperature region, a physiological temperature region and a high temperature region, and is the widest detection temperature range which can be realized at the present.