The invention relates to a
graphene aerogel-based laminated
perovskite solar cell and preparation thereof. Particularly, the preparation comprises steps: (1) after a
graphene oxide aqueous solution is taken for reduction, through vacuum
freeze drying, the
graphene aerogel is made; (2)
ethanol is added, a paste
slurry is obtained through
grinding, the paste
slurry is applied to the surface of a conductive substrate with an
oxide electron transport layer and an insulating layer, and heating
processing is carried out; (3) dispensing of a mixed
perovskite precursor solution containing lead,
iodine and / or
bromine is carried out, and annealing and cooling to a
room temperature are carried out; and (4) continuous dispensing of another mixed
perovskite precursor solution containing
tin,
iodine and / or
bromine is carried out, annealing and cooling are carried out, and preparation is completed. In comparison with the prior art, the
cell structure is simpler, two kinds of perovskite absorb different intensities of
sunlight, utilization of
solar energy is increased; and in addition, due to the use of the graphene
aerogel, the
cell cost can be reduced, the hole mobility is improved, the
cell efficiency is further enhanced, and the application prospect is wide.