The invention discloses a device and method for solution casting a large film. The device comprises a heat-preservation top cover, a stainless steel water jacket, a film casting disc, a heating plateand a heat-preservation bottom plate; the heating plate is medially arranged on the heat-preservation bottom plate, the stainless steel water jacket is arranged at the portion, wound around a round upwards, along the edge of the heat-preservation bottom plate, and is higher than the film casting disc, a condensation-solvent collecting trough is arranged at the portion, wound around a round inwards, of the bottom edge of the stainless steel water jacket, and the heat-preservation top cover covers the upper end of the stainless steel water jacket for sealing; a plurality of adjusting supportinglegs are arranged below the heat-preservation bottom plate; a plate is arranged on the upper surface of the heating plate; the film casting disc is medially arranged on the upper surface of the heating plate; float glass is arranged at the disc bottom of the film casting disc, and a round of disc edge is arranged on the edge of the disc bottom upwards; the disc bottom of the float glass of the film casting disc is in directly contact with the plate on the upper surface of the heating plate; the film casting disc is located inside the outer contour of the heating plate, and the heating plate islocated inside the outer contour of the heat-preservation bottom plate. By means of the device and method, the large-area film can be prepared, the technology is simple, the film preparing efficiencyis high, the cost is low, the crystallinity degree of a finished product film is high, the isotropy is achieved, the thickness is even, and the finished-product rate is high.