The invention discloses a
sulfide solid electrolyte based on
ionic liquid electrowetting modification and application thereof. The preparation method of the
electrolyte comprises the following steps: preparing a
sulfide electrolyte into an electrolyte sheet, and
coating the surface of the electrolyte sheet with an
ionic liquid to form an
ionic liquid film, thereby obtaining the electrolyte sheet containing the ionic liquid film; and placing the
sulfide solid electrolyte between
electrode plates which are arranged in parallel to assemble a parallel-plate
capacitor, and applying a direct-current
signal to carry out
electrowetting treatment, thereby obtaining the sulfide
solid electrolyte based on ionic liquid
electrowetting. The specific ionic liquid is introduced into the interface of the sulfide solid electrolyte and the negative
electrode for electrowetting treatment, so that the interface
contact angle is effectively reduced, the interface wettability is improved, the
interface impedance is reduced, the electrochemical performance of the all-solid-state battery is improved, and the cycle life of the all-solid-state battery is prolonged. The method particularly focuses on the use of
imidazole and
pyridine ionic liquids, and selects the appropriate ionic liquid for the
lithium metal negative
electrode material to realize the optimal interface modification effect.