The invention discloses a cross-flow internally-cooled solution dehumidifier and a method thereof. The cross-flow internally-cooled solution dehumidifier is composed of a plurality of dehumidifying units which are arranged side by side or connected in series. The dehumidifying units comprise distributive pipes, collecting pipes, capillary pipes, sleeves, liquid collecting grooves and liquid absorbing layers. The distributive pipes are provided with a plurality of capillary pipes in vertical and parallel modes, the collecting pipes are arranged at the ends of the plurality of capillary pipes, the liquid collecting grooves are arranged below the collecting pipes, the sleeves are arranged outside the distributive pipes, and one or more liquid absorbing layers are evenly and tightly wound outside each capillary pipe. Compared with the prior art, the cross-flow internally cooled solution dehumidifier and the method thereof have the advantages that first, the mass flow rate of solutions consumed by the dehumidifier is smaller than that of solutions consumed by a traditional tower type dehumidifier when moisture air with the same mass flow rate is processed; second, the air side pressure drop generated in the process of processing the moisture air is lower, the air which is processed and enters a room does not carry solution liquid drops; and third, compared with a turning wheel solid absorbing dehumidifier and a traditional liquid dehumidifier, the dehumidifier has better dehumidifying performance.