The invention relates to the field of graphene materials, particularly relates to preparation methods for graphene micro-sheets and particularly relates to a method for preparing the graphene micro-sheets by using a counter-jet jet mill. According to the method, the graphene sheets are obtained through enabling melted ferric chloride and potassium chloride to enter an interlayer of graphite, enabling the powder materials to be in collision through high-speed airflow in the counter-jet jet mill by using the characteristic of brittleness of ferric chloride and potassium chloride crystal grains and the characteristics of good fluidity and difficulty in agglomeration of talcum powder, delaminating the graphite and the talcum powder by generated impact force, shearing force and frictional force, carrying out further separation by a grading room, refluxing unqualified powder material to a crushing chamber, and yielding delaminated graphite and talcum powder as well as gas together. The continuous and large-scale production of the graphene micro-sheets, which are uniform in layer number dispersion and good in fluidity and are not prone to agglomeration, is achieved, the yield is high, the cost is low, no pollution is caused, and the layer thickness meets the requirements of use in the fields of rubber reinforcing, plastic reinforcing, coating material anticorrosion, lubrication and sewage treatment, so that the promotion of the large-scale application of graphene is facilitated.