The invention discloses a laser Raman spectrum detection method for quickly analyzing content of basic flavine in soybean hull and relates to the technical field of food detection. The laser Raman spectrum detection method includes the following steps: (1), determining basic flavine characteristic Raman peak: 650cm-1+/-3cm-1; (2), drawing a basic flavine standard curve; (3), preparing a to-be-detected sample solution; (4), taking the to-be-detected sample solution, adding nano enhanced reagent and inorganic salt flocculant, rocking uniformly, using a laser Raman spectrum instrument to detect, and acquiring a Raman spectrogram of a sample, wherein the nano enhanced reagent is one of gold, silver or copper nano sol; (5), performing qualitative determination; (6), performing quantitative determination. The laser Raman spectrum detection method has the advantages of being simple in operation and accurate, quick, lossless and low-cost in detection, is suitable for on-site emergency detection, enterprise self-control detection, large-scale sample screening detection and the like, can be used for both qualitative analysis and quantitative analysis, problematic food can be effectively recognized, and consumer rights and interests can be protected.