The invention relates to a jewel-like crystal based on animal skeletons and a preparation method of the jewel-like crystal. The preparation method comprises the following steps of burning animal skeletons into powder, then adding the powder into water, uniformly mixing, then adding an organic polymer monomer, a cross-linking agent, an initiator and a catalyst, and fully stirring to form slurry, injecting the slurry into a mold, enabling the organic polymer monomer to react, crosslink and polymerize to form polymer gel, and bonding and curing the particles in situ to form a green body, and carrying out high-temperature and high-pressure plasma-assisted sintering on the green body to obtain the jewel-like crystal. The technical means of material synthesis and crystal reconstruction are adopted, and the natural dead pet skeletons are subjected to atom recombination to form jewel-like crystals containing elements such as carbon, calcium, phosphorus, magnesium and oxygen; on the basis of the traditional hot pressing sintering technology, the plasma auxiliary sintering technology is combined, multi-field coupling of a thermal field, a force field and an electric field is achieved, energy needed by reaction is reduced, and the reaction rate and the production efficiency are improved.