The invention discloses an LED light-emitting structure, a manufacturing method thereof and a light-emitting device, the LED light-emitting structure is of a multi-layer structure, and the LED light-emitting structure sequentially comprises an LED
light source, a
grating layer, a gradient
refraction layer and a micro-
lens array layer from bottom to top; the
grating layer is used for diffracting light rays emitted by the LED
light source to the gradient
refraction layer at different angles; the gradient
refraction layer comprises a bottom refraction layer, a middle refraction layer and a top refraction layer, the refractive indexes of the bottom refraction layer, the middle refraction layer and the top refraction layer are sequentially reduced, the bottom refraction layer is connected with the
grating layer, the top refraction layer is connected with the micro-
lens array layer, and the gradient refraction layer is used for increasing the emergent angle of light; the micro-
lens array layer is used for uniformly distributing the light rays emitted by the gradient refraction layer at a larger angle; in combination with three optical structures of the grating layer, the gradient refraction layer and the micro-lens array layer, step-by-step modulation control of light is realized, functional
complementation and synergistic interaction of all the
layers are realized, the light emitting angle can be obviously increased, the light emitting uniformity can be enhanced, and in the gradient refraction layer, the
refractive index gradient can be smoothed so as to improve the light
distribution uniformity.