The invention discloses a preparation method of an LATP solid electrolyte, and relates to the technical field of lithium ion secondary battery solid electrolyte preparation, the preparation method comprises the following steps: S1, adding TiOSO4 into deionized water, mixing to prepare a TiOSO4 aqueous solution, adjusting the pH value, and preparing the TiOSO4 aqueous solution with the adjusted pH value for later use; S2, adding NaF into deionized water to prepare a NaF aqueous solution for later use; S3, adding H3PO4 into deionized water to prepare an H3PO4 aqueous solution for later use; S4, adding deionized water, NaF and H2SO4 into a reaction kettle, preparing and heating a mixed bottom water solution, adding a TiOSO4 solution, a NaF solution and a H3PO4 solution into the mixed bottom water solution at the same time, conducting solid-liquid separation, washing and drying prepared solids, and preparing Ti3 (PO4) 3 solid powder; and S5, adding an AlPO4 solid and a Li3PO4 solid into the Ti3 (PO4) 3 solid powder, mixing, sintering, crushing and sieving to obtain the LATP solid electrolyte.