The present invention relates to a flexible supercapacitor with with NiS-MoS2 heterogeneous nano-sheet array structure based on carbon cloth loading and a preparation method thereof, belonging to thetechnical field of new energy material and device preparation. The flexible supercapacitor grows high-purity, high-density and high-orientation carbon cloth-loaded NiS-MoS2 heterogeneous nanosheet array by using anode material, carbon cloth coated with activated carbon as cathode material, PVA/KOH gel as diaphragm and electrolyte respectively. The anode has the advantages of high purity, high density, tidy appearance, strict controllable growth condition, simple equipment and process, low cost, high capacitance and good charge-discharge stability. The cathode material has excellent conductivity and large double-layer capacitance. The preparation process of the capacitor is simple, economical and environmentally friendly, and no post-treatment is needed. The supercapacitor provided by the invention has the advantages of light weight, large capacity, good cycle charging and discharging stability, and good flexibility, and can be used for power supply equipment of wearable electronic devices.