An omnibearing vibration ultrasonic ball mill with high efficiency is composed of a rack, a motor, a synchronous belt wheel, a synchronous belt, an eccentric main shaft, a bearing, an eccentric wheelframe, a ball-milling tank, a ball-milling tank connecting shaft, a gas conveying pipe, an ultrasonic generator, a gas pressure sensor, a temperature sensor and an operation and control device system.One end of the eccentric wheel frame is connected with the eccentric main shaft through the bearing, and the other end of the eccentric wheel frame is connected with the ball-milling tank connectingshaft through a hinge, so that the eccentric wheel frame drives the ball-milling tank connecting shaft to swing back and forth around a fulcrum under the driving of the eccentric main shaft. The ball-milling tank connecting shaft is of a two-section structure, the section, connected with the eccentric wheel frame, of the ball-milling tank connecting shaft is a solid rod piece, the section, connected with the ball-milling tank, of the ball-milling tank connecting shaft is a hollow rod piece with high elasticity, and all connecting wires between the sensors and the operation and control device system and between the ultrasonic generator and the operation and control device system and the gas conveying pipe are led out of the ball-milling tank through the hollow rod piece, wherein the sensorsand the ultrasonic generator are arranged in the ball-milling tank.