The invention discloses supplement purely-natural mask with moisturizing, whitening and anti-wrinkle functions and a preparation method thereof; the supplement purely-natural mask comprises, by weight, 24-34 parts of pearl powder, 15-25 parts of honey, 8-13 parts of seaweed, 3-7 parts of saffron, 18-22 parts of yoghurt, 3-6 parts of carrot, 3-5 parts of olive oil, 2-6 parts of flour, 1-3 parts of shortening, and 1-3 parts of pumice; the preparation method comprises: weighing the materials according to the formula, chopping the weighed carrot into carrot paste, boiling the weighed honey at 90-100 DEG C for 3-5 min, adding the carrot paste, stirring well, adding the rest weighed materials, and mixing well. The supplement purely-natural mask can promote regeneration of skin collagen cells, effectively relieve wrinkles, relieve pigmentation of skin, provide sufficient water for the skin, and has better safety and slim chances to cause allergy as it contains no artificial synthetic chemical ingredients.