The invention discloses a
perovskite thin film, a photoelectric device and a method for improving the surface quality of the
perovskite thin film. The method for improving the surface quality of the
perovskite thin film comprises the following steps: S1, preparing the perovskite thin film; s2, performing
picosecond pulse
laser surface
polishing treatment; and S3,
guanidine ion implantation and repair: applying a
guanidine salt solution to the surface of the perovskite thin film, removing the redundant
guanidine salt solution on the surface of the perovskite thin film after the guanidine ions are implanted into the surface of the perovskite thin film, and then carrying out annealing treatment. According to the method, the surface of the perovskite thin film is polished through the
picosecond pulse
laser, the roughness of the surface of the perovskite is effectively reduced, a
surface layer rich in defects is removed, guanidine ions are selectively implanted again through a multi-A-site vacancy structure formed on the surface of the perovskite thin film subjected to
laser polishing, multiple
hydrogen bonds are formed through the guanidine ions and a perovskite framework, and the
surface roughness of the perovskite thin film is effectively reduced. And deep and stable defect
passivation and lattice strengthening are realized, and the high-quality perovskite thin film with
smooth surface, low defect density and high stability is obtained.