The invention belongs to the technical field of
photocatalysis, and particularly relates to a
graphite-phase
carbon nitride photocatalyst based on a
nitrogen-defect
sulfur-doped coupled S-type
homojunction as well as a preparation method and application of the
graphite-phase
carbon nitride photocatalyst. N-defect g-C3N4 (NA-DCN) and S-doped g-C3N4 (NA-SCN) are respectively constructed through
nitric acid assisted treatment, and directed migration of
photon-generated carriers is realized by using an S-type
homojunction interface so as to inhibit recombination; stable
interface bonding is formed through component proportion optimization, and the specific surface area and the number of active sites of the material are synchronously increased. Finally, through multi-dimensional structure regulation and control, the problems that the g-C3N4 is limited in photoresponse range, fast in carrier recombination and difficult in consideration of catalytic activity and stability are synchronously solved, the photocatalytic
hydrogen production performance of the g-C3N4 is remarkably enhanced, and a reliable technical scheme is provided for large-scale application of an efficient
carbon nitride-based photocatalytic material.