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The application relates to the technical field of nanomaterial preparation, in particular to a method for preparing Cu@Ag particles by laser, which comprises the following steps: S1, preparing a solution: dissolving a copper precursor in a solvent to obtain a copper precursor solution, and dissolving a silver precursor in a solvent to obtain a silver precursor solution; S2, irradiating the copper precursor solution by using a femtosecond pulse laser to generate nano-copper particle cores through reduction; S3, adding the silver precursor solution into the liquid phase environment containing the nano-copper particle cores, adjusting the wavelength parameter of the picosecond pulse laser to the surface of the nano-copper particle cores to realize laser energy focusing, irradiating the solution by using the picosecond pulse laser, allowing silver ions to be reduced and deposited on the surface of the nano-copper particle cores to form a silver shell, and thus obtaining Cu@Ag particles, so that the problems that the existing chemical reduction method is not environmentally friendly and it is difficult to accurately control the generation sequence of the core and the shell are solved.