The invention discloses a device assembly for manufacturing a radial tire inner liner component. The device assembly consists of a main rubber supply device, a secondary rubber supply device, a four-roll calender, a floating roll speed regulating device, an attached conveying device, a cooling device, an automatic deviation correction device, a self-shield radiation device, a rubber sheet storage device, another automatic deviation correction device, a slicing device and a double coiling device, wherein raw rubber is fed into the four-roll calender through the main rubber supply device and the secondary rubber supply device to form an inner liner component rubber sheet through calendering; the inner liner component rubber sheet enters a beam transition device in the self-shield radiation device through the attached conveying device, the cooling device and the automatic deviation correction device; the rubber sheet is irradiated through high-energy electron ray emitted by an electron accelerator; the irradiated rubber sheet gets out of transition cabins to enter the rubber sheet storage device to be tidied, is adjusted through the automatic deviation correction device, enters the slicing device to be cut and is coiled by the double coiling device for later use. The device assembly has the advantages of self-shielding function, easiness and convenience in operation, safety, convenience, stability in operation, high production efficiency, low operation cost, capability of being seamlessly connected with an inner liner calendering production line and suitability for being used in an automatic production line.