The invention discloses a preparation method for a CNT (carbon
nano tube)-SAPO (silicoaluminophosphate)-5 molecular-
sieve composite membrane. The preparation method comprises the following steps that: (1) synthetic liquid is prepared, and the
molar composition of raw materials of the synthetic liquid is that Al2O3: P2O5: SiO2: Template: H2O: X equals to 1: a: b: c: d: e, wherein a is equal to 0.8-1.3, b is equal to 0.05-1, c is equal to 0.15-1, d is equal to 45-1000, and e is equal to 0.075-0.3; (2) a porous support is put into a high-pressure
crystallization reaction kettle, the synthetic liquid is added to promote full crosslinking growth among
molecular sieve crystals, and finally, the complete
molecular sieve membrane is formed; and (3) an organic template is removed by the catalytic property of a heteroatoms-containing SAPO-5
molecular sieve. According to the invention, intergranular defects can be effectively prevented from forming in the molecular
sieve membrane, and a split organic template agent can form a CNT tube in a molecular
sieve pore passage so as to improve the hydrophobic property of the molecular sieve membrane. According to the invention, technological conditions are moderate, the operation is simpler, costs are lower, the applicability is wider, and not only is the large-scale production of molecular sieve membranes facilitated, but also the industrialized application of the molecular sieve membranes in separation of gas and separation of low-concentration organics is facilitated.